I wrote a computer program to automatically search for solutions. The first integer it couldn't find a solution for was

>! 462

Here's it's full output for all integers from 0 to 500. There are only two integers in that range it can't find solutions for. Solutions are ordered by fewest bits used, then by fewest zeros used as a tiebreaker. `s` represents square root.

    0: 0
    1: 0!
    2: 0!+0!
    3: 11
    4: 100
    5: 101
    6: 11!
    7: 11!+0!
    8: 100!!
    9: 100!!+0!
    10: 1010
    11: s(101!+0!)
    12: (11!)/.1
    13: 1101
    14: 101!!-(0!)
    15: 101!!
    16: 101!!+0!
    17: 10001
    18: (11!)*11
    19: s(((11!)!)*.1+0!)
    20: 10100
    21: 10101
    22: 100!-(0!)-(0!)
    23: 100!-(0!)
    24: 100!
    25: 100!+0!
    26: 100!+0!+0!
    27: 11^11
    28: 11100
    29: (101!!)/.1-(0!)
    30: (101!!)/.1
    31: (101!!)/.1+0!
    32: ((11!)!!)/1.1
    33: (11!)!!-(101!!)
    34: 100010
    35: (11!)^(0!+0!)-(0!)
    36: (11!)^(0!+0!)
    37: (11!)^(0!+0!)+0!
    38: s(((11!)!+0!+0!)/.1)
    39: 100!+101!!
    40: (11!)!!-(100!!)
    41: (11!)!!-(11!+0!)
    42: (11!)!!-(11!)
    43: (11!)!!-101
    44: (11!)!!-100
    45: (11!)!!-11
    46: (11!)!!-(0!+0!)
    47: (11!)!!-(0!)
    48: (11!)!!
    49: (11!)!!+0!
    50: (11!)!!+0!+0!
    51: (11!)!!+11
    52: (11!)!!+100
    53: ((11!+0!)!!+0!)*.1
    54: (11!)!!+11!
    55: (11!)!!+11!+0!
    56: ((100!!)!)/((11!)!)
    57: (11!+0!)!!-((11!)!!)
    58: (101!)*.1-(0!+0!)
    59: (101!)*.1-(0!)
    60: (101!)*.1
    61: (101!)*.1+0!
    62: (0!+0!)^(11!)-(0!+0!)
    63: (0!+0!)^(11!)-(0!)
    64: (0!+0!)^(11!)
    65: (0!+0!)^(11!)+0!
    66: (0!+0!)^(11!)+0!+0!
    67: (0!+0!)^(11!)+11
    68: s((11!+0!)!+0!)-11
    69: s((11!+0!)!+0!)-(0!+0!)
    70: s((11!+0!)!+0!)-(0!)
    71: s((11!+0!)!+0!)
    72: ((11!)!!)*1.1
    73: ((11!)!!)*1.1+0!
    74: ((11!)^(0!+0!)+0!)/.1
    75: (100!+0!)*11
    76: (s(((11!)!)*.1+0!))/.01
    77: s((11!+0!)!+0!)+11!
    78: ((11!+0!)!!-(0!))*.11
    79: (101!)/1.1-(0!)
    80: (101!)/1.1
    81: 11^100
    82: 11^100+0!
    83: 11^100+0!+0!
    84: ((11!)!!-((0!+0!+0!)!))/.1
    85: ((11!)!!-((0!+0!+0!)!))/.1+0!
    86: ((11!)!!+0!-((0!+0!+0!)!))/.1
    87: ((100!!)!!)*.1-((11!+0!)!!)
    88: ((11!)!!)/.1-(100!!)
    89: ((11!)!)*.001-(0!)
    90: ((11!)!)*.001
    91: ((11!)!)*.001+0!
    92: ((11!)!!-(0!+0!))/.1
    93: ((11!)!!-(0!))/.1-(0!)
    94: ((11!)!!-(0!))/.1
    95: ((11!)!!)/.1-(0!)
    96: ((11!)!!)/.1
    97: ((11!)!!)/.1+0!
    98: ((11!)!!+0!)/.1
    99: ((11!)!!+0!)/.1+0!
    100: ((11!)!!+0!+0!)/.1
    101: (11!+0!)!!-100
    102: (11!+0!)!!-11
    103: (11!+0!)!!-(0!+0!)
    104: (11!+0!)!!-(0!)
    105: (11!+0!)!!
    106: (11!+0!)!!+0!
    107: (11!+0!)!!+0!+0!
    108: (11!+0!)!!+11
    109: (11!+0!)!!+100
    110: (11!+0!)!!+101
    111: (11!+0!)!!+11!
    112: 101!-(100!!)
    113: (11!+0!)!!+100!!
    114: 101!-(11!)
    115: 101!-101
    116: 101!-100
    117: 101!-11
    118: 101!-(0!)-(0!)
    119: 101!-(0!)
    120: 101!
    121: 101!+0!
    122: 101!+0!+0!
    123: 101!+11
    124: 101!+100
    125: 101^11
    126: 101!+11!
    127: (0!+0!)^(11!+0!)-(0!)
    128: (0!+0!)^(11!+0!)
    129: (0!+0!)^(11!+0!)+0!
    130: ((0!+0!)^(11!)+0!)/.1
    131: ((0!+0!)^(11!)+0!)/.1+0!
    132: (100!-(0!)-(0!))*(11!)
    133: 101!-(0!)+101!!-(0!)
    134: 101!-(0!)+101!!
    135: 101!+101!!
    136: 101!+101!!+0!
    137: (100!-(0!))*(11!)-(0!)
    138: (100!-(0!))*(11!)
    139: ((11!+0!)!!)/.11-(0!)
    140: ((11!+0!)!!)/.11
    141: ((11!)!!-(0!))*11
    142: (s((11!+0!)!+0!))/.1
    143: ((11!)!!)*11-(0!)
    144: ((11!)!!)*11
    145: ((11!)!!)*11+0!
    146: ((11!)!!)*11+0!+0!
    147: ((11!)!!+0!)*11
    148: ((11!)!!+0!)*11+0!
    149: (100!+0!)*(11!)-(0!)
    150: (100!+0!)*(11!)
    151: (100!+0!)*(11!)+0!
    152: (11!+0!)!!+(11!)!!-(0!)
    153: (11!+0!)!!+(11!)!!
    154: (11!+0!)!!+(11!)!!+0!
    155: (11!+0!)!!+(11!)!!+0!+0!
    156: ((11!+0!)!!-(0!))*1.1
    157: ((11!+0!)!!-(0!))*1.1+0!
    158: (101!)/.11-(0!+0!)
    159: (101!)/.11-(0!)
    160: (101!)/.11
    161: (101!)/.11+0!
    162: (11^100)/.1
    163: (11^100)/.1+0!
    164: (11^100+0!)/.1
    165: (101!!)*(s(101!+0!))
    166: 101!-(0!)+(11!)!!-(0!)
    167: 101!-(0!)+(11!)!!
    168: 101!+(11!)!!
    169: 1101^(0!+0!)
    170: 1101^(0!+0!)+0!
    171: 1101^10+0!+0!
    172: ((11!)!)*.01-(100!!)
    173: ((11!)!)*.01-(100!!-(0!))
    174: ((11!)!)*.01-((0!+0!+0!)!)
    175: (100!+0!)*(11!+0!)
    176: ((11!)!)*.01-100
    177: ((11!)!)*.01-(0!+0!+0!)
    178: ((11!)!)*.01-(0!+0!)
    179: ((11!)!)*.01-(0!)
    180: ((11!)!)*.01
    181: ((11!)!)*.01+0!
    182: ((11!)!)*.01+0!+0!
    183: ((11!)!)*.01+0!+0!+0!
    184: ((11!)!!-(0!+0!))/.01
    185: ((11!)!!-(0!+0!))/.01+0!
    186: ((100!!)!!)*.1-(11!)
    187: ((11!)!!-(0!))/.01-(0!)
    188: ((11!)!!-(0!))/.01
    189: ((11!)!!-(0!))/.01+0!
    190: (((11!)!!)/.1-(0!))/.1
    191: ((100!!)!!)*.1-(0!)
    192: ((100!!)!!)*.1
    193: ((100!!)!!)*.1+0!
    194: (((11!)!!)/.1+0!)/.1
    195: ((11!)!!+0!)/.01-(0!)
    196: ((11!)!!+0!)/.01
    197: ((11!)!!+0!)/.01+0!
    198: ((100!!)!!)*.1+11!
    199: s((100!!)!+0!-((11!)!))
    200: ((11!)!!+0!+0!)/.01
    201: ((11!)!!+0!+0!)/.01+0!
    202: ((11!+0!)!!-100)/.1
    203: (100!!)!!-(0!)-(((11!)!)*.01)
    204: ((100!!)!!+100!)*.1
    205: ((11!+0!)!!-(0!+0!))/.1-(0!)
    206: ((11!+0!)!!-(0!+0!))/.1
    207: ((11!+0!)!!-(0!))/.1-(0!)
    208: ((11!+0!)!!-(0!))/.1
    209: ((11!+0!)!!)/.1-(0!)
    210: ((11!+0!)!!)/.1
    211: ((11!+0!)!!)/.1+0!
    212: ((11!+0!)!!+0!)/.1
    213: ((11!+0!)!!+0!)/.1+0!
    214: ((11!+0!)!!+0!+0!)/.1
    215: (11!)^11-(0!)
    216: (11!)^11
    217: (11!)^11+0!
    218: (11!)^11+0!+0!
    219: (11!)^11+0!+0!+0!
    220: ((100!!)!!+0!)/1.11
    221: (101!!)^10-100
    222: ((11!+0!)!!+(0!+0!+0!)!)/.1
    223: (101!!)^10-(0!+0!)
    224: (101!!)^(0!+0!)-(0!)
    225: (101!!)^(0!+0!)
    226: (101!!)^(0!+0!)+0!
    227: (101!!)^10+0!+0!
    228: (101!-((0!+0!+0!)!))/.1
    229: (101!!)^10+100
    230: ((11!)!!-(0!+0!))*101
    231: (101!!)^(0!+0!)+11!
    232: (101!-100)/.1
    233: (101!!)^10+100!!
    234: (101!-(0!)-(0!+0!))/.1
    235: ((11!)!!-(0!))*101
    236: (101!-(0!)-(0!))/.1
    237: (101!-(0!))/.1-(0!)
    238: (101!-(0!))/.1
    239: (101!)/.1-(0!)
    240: (101!)/.1
    241: (101!)/.1+0!
    242: (101!+0!)/.1
    243: 11^101
    244: (101!+0!+0!)/.1
    245: ((11!)!!+0!)*101
    246: (101!+0!+0!+0!)/.1
    247: (101!)/.1+100!!-(0!)
    248: (101!)/.1+100!!
    249: (101!!)^10+100!
    250: (0!+0!)^(100!!)-(11!)
    251: 10^(100!!)-101
    252: ((0!+0!)^(11!)-(0!))/.01
    253: (0!+0!)^(100!!)-11
    254: (1/.1)^(100!!)-(0!+0!)
    255: 10^(100!!)-(0!)
    256: (0!+0!)^(100!!)
    257: 10^(100!!)+0!
    258: (1/.1)^(100!!)+0!+0!
    259: (0!+0!)^(100!!)+11
    260: ((0!+0!)^(11!)+0!)/.01
    261: 10^(100!!)+101
    262: (0!+0!)^(100!!)+11!
    263: (100!!)!!-(101!+0!)
    264: (100!!)!!-(101!)
    265: (100!!)!!-(101!-(0!))
    266: (100!!)!!-(101!-10)
    267: ((11!)!)*.011-(0!+0!+0!)
    268: ((11!)!)*.011-(0!+0!)
    269: ((11!)!)*.011-(0!)
    270: ((11!)!)*.011
    271: ((11!)!)*.011+0!
    272: ((11!)!)*.011+0!+0!
    273: (101!!)^(0!+0!)+(11!)!!
    274: (101!!)^(0!+0!)+(11!)!!+0!
    275: ((11!)!!-(0!+0!))*(11!)-(0!)
    276: ((11!)!!-(0!+0!))*(11!)
    277: ((11!)!!-(0!+0!))*(11!)+0!
    278: (100!!)!!-(0!)-((11!+0!)!!)
    279: (100!!)!!-((11!+0!)!!)
    280: ((11!+0!)!!)/.011
    281: ((11!)!!-(0!))*(11!)-(0!)
    282: ((11!)!!-(0!))*(11!)
    283: ((11!)!!-(0!))*(11!)+0!
    284: (s((11!+0!)!+0!))/.01
    285: (((11!)!!)/.1-(0!))*(0!+0!+0!)
    286: ((11!)!!)*(11!)-(0!+0!)
    287: ((11!)!!)*(11!)-(0!)
    288: ((11!)!!)*(11!)
    289: ((11!)!!)*(11!)+0!
    290: ((11!)!!)*(11!)+0!+0!
    291: (((11!)!!)/.1+0!)*(0!+0!+0!)
    292: ((11!)!!+0!)*(11!)-(0!+0!)
    293: ((11!)!!+0!)*(11!)-(0!)
    294: ((11!)!!+0!)*(11!)
    295: ((11!)!!+0!)*(11!)+0!
    296: ((11!)!!+0!)*(11!)+0!+0!
    297: ((100!!)!!)*.1+(11!+0!)!!
    298: (101!)*10.1-(0!+0!)
    299: (101!)*10.1-(0!)
    300: (101!)*10.1
    301: (101!)*10.1+0!
    302: (101!)*10.1+0!+0!
    303: (100!!)!!-(11^100)
    304: (0!+0!)^(100!!)+(11!)!!
    305: (0!+0!)^(100!!)+(11!)!!+1
    306: ((11!+0!)!!+((0!+0!+0!)!)!!)/.1
    307: ((100!!)!!+1)/1.01-(0!)
    308: ((100!!)!!+0!)/1.01
    309: ((11!+0!)!!-(0!+0!))*11
    310: ((11!)!)/(0!+0!)-((11!)!!+0!+0!)
    311: ((11!)!)*.1-(0!)-(((0!+0!+0!)!)!!)
    312: ((11!)!)*.1-(((0!+0!+0!)!)!!)
    313: (100!!)!!-(s((11!+0!)!+0!))
    314: ((11!+0!)!!)*11-(0!)
    315: ((11!+0!)!!)*11
    316: ((11!+0!)!!)*11+0!
    317: ((11!+0!)!!)*11+0!+0!
    318: ((11!+0!)!!+0!)*11
    319: (101!)/.011-(0!)
    320: (101!)/.011
    321: (101!)/.011+0!
    322: ((11!)!!-(0!+0!))*(11!+0!)
    323: ((11!)*11)^(0!+0!)-(0!)
    324: ((11!)*11)^(0!+0!)
    325: ((11!)*11)^(0!+0!)+0!
    326: ((11!)*11)^(0!+0!)+0!+0!
    327: ((11!)!!-(0!))*(11!+0!)-(0!+0!)
    328: ((11!)!!-(0!))*(11!+0!)-(0!)
    329: ((11!)!!-(0!))*(11!+0!)
    330: ((11!)!!-(0!))*(11!+0!)+0!
    331: ((11!)!!-(0!))*(11!+0!)+0!+0!
    332: (100!!)!!-100-((11!)!!)
    333: (100!!)!!-1-((11!)!!+0!+0!)
    334: (100!!)!!-(0!+0!)-((11!)!!)
    335: (11!)!-(0!)-((100!!)!!)
    336: (100!!)!!-((11!)!!)
    337: (11!)!+0!-((100!!)!!)
    338: (11!)!+0!-((100!!)!!-(0!))
    339: (11!)!+0!-((100!!)!!-10)
    340: (10^(100!!)-(0!))/.11
    341: (11!+0!)^11-(0!+0!)
    342: (11!+0!)^11-(0!)
    343: (11!+0!)^11
    344: (11!+0!)^11+0!
    345: (100!-(0!))*(101!!)
    346: (11!+0!)^11+0!+0!+0!
    347: ((11!)!-(100!))*.1-(0!)
    348: ((11!)!-(100!))*.1
    349: ((11!)!-(100!))*.1+0!
    350: ((11!)!!+0!+0!)*(11!+0!)
    351: ((11!)!)*.1-(100!!+0!)
    352: ((11!)!)*.1-(100!!)
    353: ((11!)!)*.1-(0!)-((0!+0!+0!)!)
    354: ((11!)!)*.1-((0!+0!+0!)!)
    355: ((11!)!)*.1+0!-((0!+0!+0!)!)
    356: ((11!)!)*.1-100
    357: ((11!)!)*.1-(0!+0!+0!)
    358: ((11!)!)*.1-(0!+0!)
    359: ((11!)!)*.1-(0!)
    360: ((11!)!)*.1
    361: ((11!)!)*.1+0!
    362: ((11!)!)*.1+0!+0!
    363: ((11!)!)*.1+0!+0!+0!
    364: ((11!)!)*.1+100
    365: ((11!)!)*.1-(0!)+(0!+0!+0!)!
    366: ((11!)!)*.1+(0!+0!+0!)!
    367: ((11!)!)*.1+0!+(0!+0!+0!)!
    368: ((11!)!)*.1+100!!
    369: (100!!)!!-(101!!)
    370: (100!!)!!-(101!!-(0!))
    371: (100!!)!!-1101
    372: (100!!)!!-((11!)/.1)
    373: (100!!)!!-(s(101!+0!))
    374: (100!!)!!-1010
    375: (100!!)!!-1001
    376: (100!!)!!-(100!!)
    377: (100!!)!!-(11!+0!)
    378: (100!!)!!-(11!)
    379: (100!!)!!-101
    380: (100!!)!!-100
    381: (100!!)!!-11
    382: (100!!)!!-(0!+0!)
    383: (100!!)!!-(0!)
    384: (100!!)!!
    385: (100!!)!!+0!
    386: (100!!)!!+0!+0!
    387: (100!!)!!+11
    388: (100!!)!!+100
    389: (100!!)!!+101
    390: (100!!)!!+11!
    391: (100!!)!!+11!+0!
    392: (100!!)!!+100!!
    393: (100!!)!!+1001
    394: (100!!)!!+1010
    395: (100!!)!!+s(101!+0!)
    396: (100!!)!!+(11!)/.1
    397: (100!!)!!+1101
    398: (100!!)!!+101!!-(0!)
    399: (100!!)!!+101!!
    400: 10100^10
    401: 10100^10+1
    402: (100!!)!!+1001/.1
    403: (100!!)!!+s(((11!)!)*.1+0!)
    404: ((11!)!)*.1001-(0!)
    405: ((11!)!)*.1001
    406: ((11!)!)*.1001+0!
    407: (100!!)!!+100!-1
    408: (100!!)!!+100!
    409: (100!!)!!+100!+1
    410: (100!!)!!+11010
    411: (100!!)!!+100!+11
    412: ((11!+0!)!!-(0!+0!))/.01
    413: (100!!)!!-(0!)+(101!!)/.1
    414: (100!!)!!+(101!!)/.1
    415: ((11!+0!)!!-(0!))/.01-(0!)
    416: ((11!+0!)!!-(0!))/.01
    417: ((11!+0!)!!-(0!))/.01+0!
    418: (((11!+0!)!!)/.1-(0!))/.1
    419: ((11!+0!)!!)/.01-(0!)
    420: ((11!+0!)!!)/.01
    421: ((11!+0!)!!)/.01+0!
    422: (((11!+0!)!!)/.1+0!)/.1
    423: ((11!)!!-(0!))*(100!!+0!)
    424: ((11!+0!)!!+0!)/.01
    425: ((11!+0!)!!+0!)/.01+0!
    426: (s((11!+0!)!+0!))*(11!)
    427: (s((11!+0!)!+0!))*(11!)+0!
    428: ((11!+0!)!!+0!+0!)/.01
    429: (100!!)!!-1+(11!)!!-(0!+0!)
    430: (100!!)!!-(0!+0!)+(11!)!!
    431: (100!!)!!-(0!)+(11!)!!
    432: (100!!)!!+(11!)!!
    433: (100!!)!!+0!+(11!)!!
    434: (100!!)!!+0!+0!+(11!)!!
    435: (100!!)!!+10+(11!)!!+0!
    436: (100!!)!!+100+(11!)!!
    437: (100!!)!!+((11!+0!)!!+0!)*.1
    438: (100!!)!!+(11!)!!+(10+0!)!
    439: ((100!!)!!+0!)/.111-(0!)
    440: ((100!!)!!+0!)/.111
    441: 10101^(0!+0!)
    442: 10101^10+0!
    443: (100!!)!!+(101!)*.1-(0!)
    444: (100!!)!!+(101!)*.1
    445: (100!!)!!+(101!)*.1+0!
    446: ((101!!)^10-(0!+0!))/.1
    447: (100!!)!!-1+(0!+0!)^(11!)
    448: (100!!)!!+(0!+0!)^(11!)
    449: ((11!)!)*.101-(0!)
    450: ((11!)!)*.101
    451: ((11!)!)*.101+0!
    452: ((101!!)^(0!+0!)+0!)/.1
    453: ((11!)!)*.101+0!+0!+0!
    454: (100!!)!!-(0!)+s(111!+0!)
    455: (100!!)!!+s((11!+0!)!+0!)
    456: (100!)*(s(((11!)!)*.1+0!))
    457: ((11!)!)*.1+0!+(((0!+0!+0!)!)!!)/.1
    458: (((0!+0!+0!)!)!)*.1+((11!)!!+0!)/.1
    459: ((11!+0!)!!+(11!)!!)*(0!+0!+0!)
    460: ((11!)!!-(0!+0!))*1010
    461: (((11!)!!)^(0!+0!)+0!)/101
    462 was not found
    463: (11!)!-(0!)-(10^(100!!))
    464: (11!)!-((0!+0!)^(100!!))
    465: ((11!)!)*.1+((0!+0!+0!)!+0!)!!
    466: ((11!)!)*.1+(100!!-(0!))!!+0!
    467: ((100!!+0!)!!+0!)*.1-(11!)
    468: (101!-(0!)-10)/.01
    469: ((11!)!!-(0!))*1010-(0!)
    470: ((11!)!!-(0!))*1010
    471: (1001!!-(0!))*.1-(0!)
    472: ((100!!+0!)!!-(0!))*.1
    473: ((100!!+0!)!!+0!)*.1
    474: (1001!!+0!)*.1+0!
    475: (101!-(0!))/.01-(0!)
    476: (101!-(0!))/.01
    477: (101!-(0!))/.01+0!
    478: ((101!)/.1-(0!))/.1
    479: ((11!)!)/1.1-(0!)
    480: ((11!)!)/1.1
    481: ((11!)!)/1.1+0!
    482: ((11!)!)/1.1+0!+0!
    483: (101!+0!)/.01-(0!)
    484: (101!+0!)/.01
    485: (101!+0!)/.01+0!
    486: ((0!+0!+0!)^101)/.1
    487: (100!!)!!-(0!+0!)+111!!
    488: (100!!)!!-(0!)+(11!+0!)!!
    489: (100!!)!!+(11!+0!)!!
    490: (100!!)!!+0!+(11!+0!)!!
    491: (100!!)!!+10+(11!+0!)!!
    492: ((11!)!)*.11-(((0!+0!+0!)!)!!)
    493: ((11!)!-(0!))/.1-((100!!+0!)!!)
    494: (11!)!-(0!)-((101!!)^(0!+0!))
    495: (((0!+0!+0!)!)!)*.1011
    496: (101!+100)/.01
    497: (s((11!+0!)!+0!))*(11!+0!)
    498: ((11!)!)*.101+((0!+0!+0!)!)!!
    499 was not found
    500: (1010^11)/(0!+0!)

The solver can be found here: https://github.com/isaacg1/eight-bits/

Caveats:
* The solver does not consider intermediate steps with value above 65535.

* The solver does not consider intermediate steps with negative value. I believe intermediate steps with negative value should never be necessary.

* The solver does not consider intermediate steps with fractional value. Literals with fractional value are used, but intermediate steps with fractional value are not.

I believe that my solver finds all possible solutions that do not go through one of the above three cases.