Their ages are:
71, 9, 4$71, 9, 4$
Reasoning:
The oldest grandchild's age is (presumably) a perfect square, and the square of her age is 10$10$ years older than a reasonable grandma age, so we can guess that she is now 9$9$. That makes the grandma 71$71$, and the younger child is 4$4$. So thus the grandma was 64$64$ when she was diagnosed.